MSE Colloquium: Lauren Garten, Enhancing Converse Magnetoelectric Coupling Through Strain Engineering in Artificial Multiferroic Heterostructures

Assistant Professor, School of Materials Science and Engineering, Georgia Institute of Technology

Abstract

Magnetoelectric materials present a unique opportunity for electric field-controlled magnetism. Even though strain mediated multiferroic heterostructures have shown unprecedented magnetoelectric coupling compared to single phase materials, further improvement must be made before ultra-low power memory, logic, magnetic sensors, and wide spectrum antennas can be realized. Here, we describe how magnetoelectric coupling can be enhanced by simultaneously exploiting multiple strain engineering approaches. This work is conducted on heterostructures composed of Fe0.5Co0.5/Ag multilayers on (011) Pb(In1/2Nb1/2)O3–Pb(Mg1/3Nb2/3)O3–PbTiO3 piezoelectric crystal substrates. When grown and measured under strain these heterostructures exhibit an effective converse magnetoelectric coefficient on order of 10-5 s/m: the highest directly measured, non-resonant value to-date. Additionally, this response occurred at room temperature and at low electric fields (< 2 kV/cm). This large effect is enabled by the magnetization reorientation caused by changing the magnetic anisotropy with strain from a piezoelectric phase transition and the use of multilayered magnetic materials to minimize the internal stress from deposition. Additionally, the coercive field dependence of the magnetoelectric response under strain suggests contributions from a domain-mediated magnetization switching modified by the voltage-induced magnetoelastic anisotropy. This work highlights how multicomponent strain engineering enables enhanced magnetoelectric coupling in heterostructures and provides an approach to realize new energy efficient magnetoelectric applications.

Bio

Lauren Garten started as an assistant professor in Materials Science and Engineering at the Georgia Institute of Technology starting in the fall of 2021. Prior to that, she was a staff scientist at the U.S. Naval Research Lab (NRL) working on the growth and characterization of novel piezoelectric and artificial multiferroic heterostructures for sensors and electronics. Her work at NRL was supported by the Jerome and Isabella Karle Distinguished Fellowship and a National Research Council Associateship. Prior to this, she was a staff scientist in ferroelectric metrology development at Sandia National Laboratory and a post-doc at the National Renewable Energy Laboratory (NREL) where she worked on the processing and characterization of metastable photovoltaic materials. She received her Ph.D. in material science from the Pennsylvania State University with Prof. Susan Trolier-McKinstry on the development of piezoelectric and ferroelectric materials for tunable dielectrics. And her bachelors is in ceramic engineering from the Missouri University of Science and Technology. She has won the AFOSR Young Investigator Award, the DOE-BES Postdoctoral Research Award, the Outstanding Mentor Award from NREL, and the CalTech Young Investigator Lectureship. Her work focuses on the development of multifunctional multiferroics for energy and electronic applications, particularly at the nexus between ferroelectricity, magnetism, and photovoltaics.